Many-body effect of mesoscopic localized states in MoS 2 monolayer
2019
Transition-metal dichalcogenide monolayers provide an emerging material system to implement quantum photonics with intrinsic two-dimensional excitons or embedded zero-dimensional localized states. Here, we demonstrate mesoscopic localized states between two and zero dimensions, which is a many-body system with electron-electron Coulomb interactions. A fine-structure splitting is observed, which is similar to quantum dots. Meanwhile, the polarization degree is changed by the magnetic field, due to the nature of the two-dimensional monolayers. Furthermore, a large quadratic diamagnetism with a coefficient of around $100\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}\mathrm{eV}/{\mathrm{T}}^{2}$ is observed, as a unique consequence of the mesoscopic scale. The many-body effect also results in the emission energy variation and linewidth narrowing in the spectrum, which corresponds well to the theoretical analysis. These unique properties indicate the great potential of mesoscopic localized states in many-body physics and quantum photonics.
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