Investigating the Utility of Hyperspectral Sounders in the 9.6 μm Band to Improve Ozone Analyses

Currently, hyperspectral sounder brightness temperatures assimilated in the Goddard Earth Observing System - Atmospheric Data Assimilation System (GEOS-ADAS) are limited to assimilating temperature and moisture. The ozone sensitive 9.6 micron region is sensed by several hyperspectral sounders including AIRS (Atmospheric InfraRed Sounder), IASI (Infrared Atmospheric Sounding Interferometer), and CrIS (Cross-track Infrared Sounder). Direct assimilation of brightness temperatures in the 9.6 micron region have been used previously to improve ozone analyses. This has recently been achieved by ECMWF (European Centre for Medium-Range Weather Forecast) (Dragani and McNally, 2013; Eresmaa et al., 2017), and while every system presents its challenges, it should be possible to take advantage of this spectral region using the GEOS-ADAS. For this study, channels were selected from available operational subsets evaluating information content, and minimizing inter-channel correlation. Additionally, information such as channel selections made by other studies, and vertical sensitivities of ozone and temperature were considered in developing the study. The analyses produced show improvements verified against ozonesondes taken from SHADOZ (Southern Hemisphere Additional Ozonesondes), and WOUDC (World Ozone and Ultraviolet Data Center). The addition of ozone channels does degrade forecast skill in the Tropics, on the border of statistical significance. Overall, the addition of these channels in some form could improve ozone analyses in the GEOS-ADAS.