Assessment of pre-industrial to present-day anthropogenic climate forcing in UKESM1

Abstract. Quantifying forcings from anthropogenic perturbations to the Earth System (ES) is important for understanding changes in climate since the pre-industrial period. In this paper, we quantify and analyse a wide range of present-day (PD) anthropogenic climate forcings with the UK's Earth System Model (ESM), UKESM1, following the protocols defined by the Radiative Forcing Model Intercomparison Project (RFMIP) and the Aerosol and Chemistry Model Intercomparison Project (AerChemMIP). In particular, by quantifying effective radiative forcings (ERFs) that include rapid adjustments within a full ESM, it enables the role of various climate-chemistry-aerosol-cloud feedbacks to be quantified. Global mean ERFs are 1.83, 0.13, −0.33, and 0.93 W m−2 at the PD (Year 2014) relative to the pre-industrial (PI; Year 1850) for carbon dioxide, nitrous oxide, ozone-depleting substances, and methane, respectively. The PD total greenhouse gas ERF is 2.89 W m−2, larger than the sum of the individual GHG ERFs. UKESM1 has an aerosol forcing of −1.13 W m−2. A relatively strong negative forcing from aerosol-cloud interactions and a small negative instantaneous forcing from aerosol-radiation interactions are partially offset by a substantial forcing from black carbon absorption. Internal mixing and chemical interactions mean that neither the forcing from aerosol-radiation interactions nor aerosol-cloud interactions are linear, making the total aerosol ERF less than the sum of the individual speciated aerosol ERFs. Tropospheric ozone precursors, in addition to exerting a positive forcing due to ozone, lead to oxidant changes which in turn cause an indirect aerosol ERF, altering the sign of the net ERF from nitrogen oxide emissions. Together, aerosol and tropospheric ozone precursors (near-term climate forcers, NTCFs) exert a global mean ERF of −1.12 W m−2, mainly due to changes in the cloud radiative effect. There is also a negative PD ERF from land use (−0.32 W m−2). It is outside the range of previous estimates, and is most likely due to too strong an albedo response. In combination, the net anthropogenic ERF is potentially biased low (1.61 W m−2) relative to other estimates, due to the inclusion of non-linear feedbacks and ES interactions. By including feedbacks between greenhouse gases, stratospheric and tropospheric ozone, aerosols, and clouds, some of which act non-linearly, this work demonstrates the importance of ES interactions when quantifying climate forcing. It also suggests that rapid adjustments need to include chemical as well as physical adjustments to fully account for complex ES interactions.